Bioenergetics and Thermodynamics: Model Systems: Synthetic by A. Braibanti (auth.), A. Braibanti (eds.)

By A. Braibanti (auth.), A. Braibanti (eds.)

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Extra resources for Bioenergetics and Thermodynamics: Model Systems: Synthetic and Natural Chelates and Macrocycles as Models for Biological and Pharmaceutical Studies

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A detailed Ni(II)-binding studies were undertaken with these chelating agents with a view to understand the reason for their efficiency in the removal of Ni(II). 1. INTRODUCTION Metal toxicity caused by excessive intake of metal due to occupational exposure or environmental pollution is of much concern in recent years. There are reports of high level of Ni(II) in the blood of individuals in the mining town of Sudbury, Ontario, the site of the largest open-pit nickel mines in North America (1). The results showed that the serum nickel in the healthy inhabitants of Sudbury was double that of healthy inhabitants of Hartford, Connecticut, a city with relatively low environmental concentration of nickel.

In (~), the stronger hydrogen bonding potential of a pyridyl nitrogen is demonstrated by its high Ka value relative to that for (~). 3. HANDEDNESS AND SYMMETRY Chirality can be introduced into synthetic receptor molecules in one of two ways. Resolution of a racemic modification of an appropriate synthon provides one approach to the problem. The other approach - which will be illustrated here - is to incorporate natural products into the syntheses of the receptor molecules. The most obvious way to render the crown ether binding sites chiral is to employ readily available enantiomerically pure carbohydrates with known chiroptical properties in their syntheses.

P. : 1973, Structure and Bonding 16, p. 1. : 1977, Pure Applied Chern. 49, p. 857. : 1978, Pure Applied Chern. 50, p. 871. : 1978, Accounts Chern. Res. 11, p. 49. : 1975, Pure Applied Chern. 43, pp. 327-349. S. Chern. , p. 481 and references cited therein. : 1967, J. Arn. Chern. Soc. 89, p. 2495, 7017. : 1972, Angew. Chern. 84, p. 16 and references cited therein. : 1973, Tetrahedron 29, p. 1629. S. Chern. , p. 1055. S. Chern. , p. 15. : 1976, Helv. Chirn. Acta 59, p. 1566. S. Chern. , p. 393. : 1976, Heterocycles 5, p.

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